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Development of an electrospray photoelectron spectroscopy apparatus with a low temperature ion trap.


EMSL Project ID
3170

Abstract

We propose to develop an electrospray photodetachment apparatus with a low temperature ion trap. We have pioneered photoelectron spectroscopic studies of multiply charged anions and solution species in the gas phase using electrospray ionization (ESI). A critical feature of this apparatus is its ability to trap ions and accumulate number density from the CW ESI source for subsequent TOF mass analyses. A low temperature trap will be critical to suppress thermal broadening in the PES spectra and help stabilize weakly bound clusters. Other novel features of the proposed apparatus include pre-mass selection before the ion trapping and a high resolution reflectron TOM mass spectrometer. The new apparatus will be the first prototype of a low-temperature ion trap, which will have major impact in the filed of ion spectroscopy and physical chemistry.

Project Details

Project type
Exploratory Research
Start Date
2002-12-04
End Date
2005-12-11
Status
Closed

Team

Principal Investigator

Lai-Sheng Wang
Institution
Brown University

Team Members

Xuebin Wang
Institution
Pacific Northwest National Laboratory

Hin-koon Woo
Institution
The Scripps Research Institute

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