Skip to main content

Exploring the Radiation Damage Resistance of Nanoscale Interfaces


EMSL Project ID
46001

Abstract

The objective of this research is to rigorously test the hypothesis that internal interfaces can be manipulated at the nanoscale to enhance recombination of radiation-produced defects to dramatically reduce radiation damage without compromising other physical and mechanical properties. This hypothesis has never been rigorously tested and there has never been a fundamental study of radiation damage at interfaces that encompasses the wide range of interface types and structures proposed here. In this project we seek to 1) understand defect absorption at interfaces as a function of interface character and properties, 2) determine interface ability to adsorb and delocalize defects to promote recombination, and 3) determine interface stability and evolution under irradiation, including the saturation limit for defect absorption. This proposal is aligned with two of the principal focus areas within the Materials Sciences and Engineering Division of BES; including exploration of approaches to improve materials performance through interfacial design, and investigation of radiation effects on the mechanical and physical behavior of materials. The work consists of integrated experiments and modeling of a wide range of interface types to determine how variation in interface properties can affect defect absorption and recombination. Precisely tailored interfaces as well as nanostructured polycrystalline thin films will be studied in order to explore the full range of interface types relevant to the materials found in advanced nuclear energy systems. Reaching these objectives will demonstrate the stated hypothesis by determining interface stability under irradiation and will enable design of higher performance nuclear energy systems with attendant economic, safety and environmental benefits.

Project Details

Project type
Exploratory Research
Start Date
2011-12-27
End Date
2013-02-12
Status
Closed

Team

Principal Investigator

Richard Kurtz
Institution
Pacific Northwest National Laboratory

Team Members

Brian Wirth
Institution
University of Tennessee

Howard Heinisch
Institution
Pacific Northwest National Laboratory

Amity Andersen
Institution
Environmental Molecular Sciences Laboratory

Vaithiyalingam Shutthanandan
Institution
Environmental Molecular Sciences Laboratory

Chongmin Wang
Institution
Environmental Molecular Sciences Laboratory

Tiffany Kaspar
Institution
Pacific Northwest National Laboratory

Alan Joly
Institution
Pacific Northwest National Laboratory

Renee Van Ginhoven
Institution
Pacific Northwest National Laboratory

Related Publications

Kaspar TC, ME Bowden, CM Wang, V Shutthanandan, S Manandhar, RM Van Ginhoven, BD Wirth, and RJ Kurtz. 2013. "Defect Structure of Spitaxial CrV Thin Films on MgO(001)." Thin Solid Films 550:1-9. doi:10.1016/j.tsf.2013.09.067