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Linear-response, real-time electron dynamics & high-level excited-state properties of molecules and materials


EMSL Project ID
46003

Abstract

This is a three-pronged proposal aimed to address excited state properties in molecules and materials using linear-response TDDFT, real-time electronic dynamics and high-level coupled cluster approaches. This effort will be a combination of development and application with three distinct and simultaneous thrusts: development of the functionality within the NWChem framework; collaboration with ongoing spectroscopy experiments at EMSL; and exploratory computational experiments to address ongoing mysteries and to act as a driver for new experiments at EMSL.

Project Details

Start Date
2011-10-04
End Date
2012-10-07
Status
Closed

Team

Principal Investigator

Niranjan Govind
Institution
Pacific Northwest National Laboratory

Team Members

Shaul Mukamel
Institution
University of California, Irvine

Micah Prange
Institution
Pacific Northwest National Laboratory

Kenneth Lopata
Institution
Louisiana State University

Marat Valiev
Institution
Environmental Molecular Sciences Laboratory

Renee Van Ginhoven
Institution
Pacific Northwest National Laboratory

Related Publications

Lopata KA, BE Van Kuiken, M Khalil, and N Govind. 2012. "Linear-response and real-time time-dependent density functional theory studies of core-level near-edge x-ray absorption." PNNL-SA-88981, Pacific Northwest National Laboratory, Richland, WA.
Zhang Y, JD Biggs, D Healion, N Govind, and S Mukamel. 2012. "Core and Valence Excitations in Resonant X-ray Spectroscopy using Restricted Excitation Window Time-dependent Density Functional Theory." Journal of Chemical Physics 137(19):Article No. 194306. doi:10.1063/1.4766356