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Valence and Core-Level Excited State Spectroscopy and Dynamics and Magnetic Resonance Spectroscopy Studies of Molecules and Materials in Complex Environments


EMSL Project ID
49115

Abstract

This is a multi-pronged proposal aimed at theoretical developments and modeling of a variety of spectroscopies (UV/Vis, XAS, EELS, NMR, EPR, Raman), ultrafast electron (de)localization dynamics and charge transfer and transport in photoactivated processes. This effort will be a combination of development and application with four thrusts: development of the functionality within the NWChem framework; collaboration with ongoing spectroscopy experiments at EMSL and EMSL users; and exploratory computational experiments to act as a driver for new experiments at EMSL and PNNL; and state-of-the-art X-ray spectroscopies at DOE light sources.

Project Details

Start Date
2015-10-15
End Date
2016-09-30
Status
Closed

Team

Principal Investigator

Niranjan Govind
Institution
Pacific Northwest National Laboratory

Team Members

Amity Andersen
Institution
Environmental Molecular Sciences Laboratory

Jacek Jakowski
Institution
Oak Ridge National Laboratory

Related Publications

Ueltschi TW, SA Fischer, E Apra, AN Tarnovsky, N Govind, PZ El-Khoury, and WP Hess. 2016. "Time-Domain Simulations of Transient Species in Experimentally Relevant Environments." Journal of Physical Chemistry A 120(4):556-561. doi:10. 1021/acs. jpca. 5b11710