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The electronic structure and dynamics of photocatalytic and electronic interfaces


EMSL Project ID
13894b

Abstract

IThe electronic structure of unoccupied states and defects represents one of the most experimentally and theoretically demanding challenges in the science of interfacial phenomena. Here we propose a joint theoretical and experimental study on the photocatalytic and electronic properties of molecule-metal oxide and molecule-metal interfaces. Particularly, we will focus on the electronic structure and charge transfer dynamics of H2O covered TiO2 surfaces. We will explore the wet electron states in H2O overlayers on epitaxial anatase TiO2 films by time-resolved photoemission and DFT theory. The knowledge gained on water covered TiO2 will have broad relevance to charge transfer driven phenomena at environmental interfaces. In addition, we will study the superatom electronic properties of endohedrally doped fullerenes and related materials.

Project Details

Project type
Large-Scale EMSL Research
Start Date
2008-08-19
End Date
2011-09-30
Status
Closed

Team

Principal Investigator

Hrvoje Petek
Institution
University of Pittsburgh

Team Members

Hongli Guo
Institution
California State University, Northridge

Hao Sun
Institution
University of Pennsylvania

Huijuan Sun
Institution
University of Science and Technology of China, Chinese Academy of Sciences

Xuefeng Cui
Institution
University of Pittsburgh

Qijing Zheng
Institution
University of Science and Technology of China, Chinese Academy of Sciences

Chungwei Lin
Institution
University of Pittsburgh

Wissam Al-Saidi
Institution
University of Pittsburgh

Jin Zhao
Institution
University of Science and Technology of China, Chinese Academy of Sciences

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