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Molecular Interactions and Dynamics at Solid Electrolyte Interfaces


EMSL Project ID
40125

Abstract

We will carry out a systematic study on molecular interactions and dynamics at solid electrolyte interfaces (SEIs) of Li-ion batteries using primarily in situ quantitative nonlinear optical spectroscopy measurements. The objectives of this study are 3 fold: (1) to establish molecular-level metrology for characterizing SEI structures and compositions in situ; (2) to unravel molecular mechanisms governing the reactivity and interactions of various molecules at the interface; (3) to develop quantitative metrics for assessing the performance of Li-ion battery via in situ measurements. Furthermore, a general theoretical framework will be developed and validated on the basis of quantitative measurements. Combined experimental and theoretical studies of the basic materials systems will cast new insights in molecular interaction and reactivity at electrode/electrolyte interfaces, which will be critical for the design and development of next generation batteries. This study aligns with the EMSL scientific theme of Science of Interfacial Phenomena, specifically, 'In situ real-time investigations of dynamical processes at surfaces or interfaces'. EMSL's state of the art measurement capability, particularly the nonlinear optical spectroscopy, provides the only feasible means for the proposed study.

Project Details

Project type
Large-Scale EMSL Research
Start Date
2010-10-06
End Date
2013-09-30
Status
Closed

Team

Principal Investigator

Howard Wang
Institution
State University of New York at Binghamton

Team Members

Priyanka Bhattacharya
Institution
University of Dayton Research Institute

Hui Zhan
Institution
Wuhan University

Xilin Chen
Institution
Pacific Northwest National Laboratory

Liwen Ji
Institution
Pacific Northwest National Laboratory

Meng Gu
Institution
Pacific Northwest National Laboratory

Jie Xiao
Institution
University of Arkansas, Fayetteville

Xiaolin Li
Institution
Pacific Northwest National Laboratory

Hongfei Wang
Institution
Fudan University

Wu Xu
Institution
Pacific Northwest National Laboratory

Jiguang Zhang
Institution
Pacific Northwest National Laboratory

Yuyan Shao
Institution
Pacific Northwest National Laboratory

Jun Liu
Institution
Yale University

Yongsoon Shin
Institution
Pacific Northwest National Laboratory

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