Projects

Dissecting bacterial heterogeneity using fluorescence and imaging mass spectrometry

Lead Institution

University of Massachusetts Medical School

Principal Investigator

Elizabeth Shank

Project type

Exploratory Research

In nature, most microbes exist as members of complex multispecies communities that play vital roles promoting plant and soil health. Many of these microbial communities exist as biofilms: structured…

Investigation of morphological and mixing state properties of aerosol and ice crystal residual particles from the Atlantic sector of the Arctic

Lead Institution

West Texas A&M University

Principal Investigator

Seong-gi Moon

Project type

Exploratory Research

Our current knowledge of aerosol-cloud interactions in the Arctic is inadequate for accurate modeling of northern high-latitude regions. To fill this gap, the field campaign was recently conducted in…

Large Eddy Simulation of Turbulence at the Sediment-Water Interface

Lead Institution

Oregon State University

Principal Investigator

Sourabh Apte

Project type

Exploratory Research

Understanding the fundamental connections between surface and groundwater is a critical component of the current PNNL Subsurface Science Scientific Focus Area (SFA). The sediment-water interface in…

Evaluating the role of carbon radicals on Photocatalytic Nitrogen Fixation on Titania

Lead Institution

Georgia Institute of Technology

Principal Investigator

Marta Hatzell

Project type

Exploratory Research

Photocatalytic fixation of nitrogen by titania catalysts at ambient conditions has been reported for decades, yet the active site capable of adsorbing an inert N2 molecule at ambient pressure and the…

Theoretical study of photoreduction of CO2 on TiO2 surface

Lead Institution

University of Science and Technology of China, Chinese Academy of Sciences

Principal Investigator

Jin Zhao

Project type

Exploratory Research

The efficient photoreduction of carbon dioxide to a fuel is a major hurdle in the neutral energy cycle of CO2, and TiO2 is one of the most intensively studied photocatalytic materials for CO2…

Integration of Omics into a New Comprehensive Rate Law for Competitive Terminal Electron-Accepting Processes in Reactive Transport Models: Application to N, Fe, S, and Contaminant Transformations in Stream and Wetland Sediments

Lead Institution

Georgia Institute of Technology

Principal Investigator

Frank Stewart

Project type

Exploratory Research

We recently received notification that our DOE-BER proposal (ID: 0000231737, Program Manager: Paul Bayer) was funded to define a new comprehensive rate law for metabolic processes in freshwater…

Understanding the long-term fate of nitrate in terrestrial ecosystems: Organic N species

Lead Institution

Cornell University

Principal Investigator

Carmen Martinez

Project type

Exploratory Research

We propose a series of experiments aimed at elucidating the mechanisms associated with the incorporation of nitrate (NO3-) into soil organic matter (SOM), with broad implications for the N…

Fate of Cosmetic Microbeads and Silver Nanoparticles in Soils

Lead Institution

Washington State University

Principal Investigator

Markus Flury

Project type

Large-Scale EMSL Research

Plastic microbeads and silver nanoparticles contained in cosmetic and health care products usually end up in our household waste water, which will then be treated in a waste water treatment plant…

Computational Studies of Catalyzed Chemical Transformations of Biomass and Derived Intermediates

Lead Institution

University of Alabama

Principal Investigator

David Dixon

Project type

Large-Scale EMSL Research

There is a critical need to develop new, renewable sources of energy as well as feedstocks for the chemical industry. Biomass is a carbon neutral source of energy and can also address issues related…

First principles investigations on the coupling of polaron and excited carrier dynamics at TiO2/molecule interface

Lead Institution

University of Pittsburgh

Principal Investigator

Hrvoje Petek

Project type

Large-Scale EMSL Research

We propose to perform computational studies of the structure and dynamics of polarons in TiO2 and related materials. The nature of charge carriers in photocatalytic semiconductors is crucial to their…

Comprehensive Characterization of the Cellulosomes from Anaerobic Gut Fungi

Lead Institution

University of California, Santa Barbara

Principal Investigator

Michelle O'Malley

Project type

Large-Scale EMSL Research

This proposal seeks use of EMSL resources to characterize the secreted, multi-enzyme cellulosomes that originate from anaerobic gut fungi. Cellulosomes enable anaerobic fungi to tether different…

Improving the accuracy and reliability of Earth system reconstructions by quantifying mechanisms that modulate sub-micron heterogeneity in marine calcifiers

Lead Institution

Oregon State University

Principal Investigator

Jennifer Fehrenbacher

Project type

Large-Scale EMSL Research

Reconstructions of Earth's biogeochemical history, the interactions between the ocean, atmosphere, and global environmental conditions, are commonly based on reconstructions generated using…

Developing a Modular Scaffold to Drive the Symmetric Assembly of Cellular Proteins for Single Particle Cryo-EM Imaging

Lead Institution

University of California, Los Angeles

Principal Investigator

Todd Yeates

Project type

Large-Scale EMSL Research

High resolution structural studies can provide exceptionally valuable information on the workings of cellular components and molecular machines, many of which play critical roles in biological energy…

The Transformation of Tetrahedral to Octahedral Coordination in Anions of Interest in High-Level Tank Waste

Lead Institution

Pacific Northwest National Laboratory

Principal Investigator

Jian-zhi Hu

Project type

Large-Scale EMSL Research

We propose to use nuclear magnetic resonance (NMR), Raman and Fourier transform-infrared (FT-IR) spectroscopy in combination with computational modeling to study the conversion of soluble tetrahedral…

System Approaches to Study Soybean Root Biology at Single-Cell Resolution

Lead Institution

University of Missouri - Columbia

Principal Investigator

Gary Stacey

Project type

Large-Scale EMSL Research

The long-term goal of this project is to further basic understanding of the agronomically important Bradyrhizobium japonicum-soybean nitrogen fixing symbiosis. Soybeans are the major source of…

Implications of U(IV)-silicate core-shell colloids for radionuclide transport

Lead Institution

University of Manchester

Principal Investigator

Samuel Shaw

Project type

Large-Scale EMSL Research

Here we will use a range of techniques to advance fundamental and predictive understanding of uranium colloids in the subsurface environment. Recent work has highlighted that U(IV)-silicate colloids…

Characterizing the functional transition of endophytic fungi during plant senescence

Lead Institution

University of California, Santa Barbara

Principal Investigator

Ryoko Oono

Project type

Large-Scale EMSL Research

Decomposition of leaf litter by a diverse microbial community is a major biogeochemical process in the global carbon cycle. Fungi are considered the primary decomposers of plant litter, especially of…

Wet Non-Aqueous Supercritical Fluid Interactions with Densified Model Rock Materials

Lead Institution

St. Mary's College of Maryland

Principal Investigator

Geoffrey Bowers

Project type

Large-Scale EMSL Research

Our research program investigates the fundamental molecular-scale dynamics, energetics, and reactivity of geochemically relevant solid-fluid interfaces by integrating experimental spectroscopy and…

Fluxomics-based elucidation of metabolic remodeling and optimization strategies for enhancing bioproduction efficiency in microbial factories under selection pressure

Lead Institution

University of Maryland, College Park

Principal Investigator

Daniel Dwyer

Project type

Large-Scale EMSL Research

Well characterized bacterial models such as Escherichia coli are ubiquitously used as microbial factories in the commercial production of biofuels and bioproducts. The increasingly optimized…

The persistence of soil organic carbon in the mineralosphere as a function of the soil microbiome, proteome, and exometabolome

Lead Institution

University of California, Berkeley

Principal Investigator

Mary Firestone

Project type

Large-Scale EMSL Research

Soils store more carbon (C) than the atmosphere and biosphere combined, yet the fundamental mechanisms that regulate the persistence of this vast pool of C remain elusive. Soil organic matter (SOM)…