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Nuclear Processing
Science Initiative


EMSL Project ID
49654

Abstract

The Nuclear Process Science Initiative (NPSI) is an internal, Laboratory Directed Research and Development (LDRD) program investment in support of the nuclear science and technology research enterprise at the Pacific Northwest National Laboratory (PNNL). This five-year investment is intended to build expertise and capabilities in nuclear materials characterization, chemistry, physics, and engineering to support capture of business opportunities in legacy waste management and nuclear nonproliferation.
The science vision for NPSI is to understand, harness, and exploit the interfacial phenomena controlling the behavior of materials in post reactor nuclear fuel processing. Research activities in support of this vision will be focused into the following Science Thrusts:

1. Interfacial Chemistry and Physics: Understand and harness the chemical and physical driving forces controlling solid phase formation, agglomeration, and dissolution in harsh environments.
2. Chemical fractionation: Discover and exploit the chemical and physical driving forces controlling the formation, distribution and influence of trace species during the processing of nuclear materials.
3. Multi-scale Modeling: Anticipate problems and signatures in post reactor nuclear fuel processing using validated multi-scale models representing relevant chemical and physical driving forces.

NPSI will strengthen PNNL’s nuclear materials capabilities, including advanced characterization, analytics, and handling, to enhance the capture of client funding to support these critical mission areas. In the legacy waste management area, NPSI will create the foundation and demonstrate our ability to understand, predict, and control tank waste behavior in key areas and with the level of confidence required to substantially reduce cost in the current baseline. This initiative will also enable development of, as well as facilitate, transformational alternatives for legacy waste processing. In nonproliferation, NPSI will demonstrate our ability to discover and develop new process signatures in nuclear materials and provide the basis for PNNL to host a laboratory-scale nuclear reprocessing capability. This capability will support a variety of research and development (R&D) of high interest to national security clients, substantially enhancing the nation’s ability to combat nuclear proliferation and terrorism.

Project Details

Start Date
2016-10-14
End Date
2017-09-30
Status
Closed

Team

Principal Investigator

Sue Clark
Institution
Pacific Northwest National Laboratory

Team Members

Dallas Reilly
Institution
Pacific Northwest National Laboratory

Jon Schwantes
Institution
Pacific Northwest National Laboratory

Jaehun Chun
Institution
Pacific Northwest National Laboratory

Sebastien Kerisit
Institution
Pacific Northwest National Laboratory

Ram Devanathan
Institution
Pacific Northwest National Laboratory

Eugene Ilton
Institution
Pacific Northwest National Laboratory

Edgar Buck
Institution
Pacific Northwest National Laboratory

Gregg Lumetta
Institution
Pacific Northwest National Laboratory

Related Publications

Peterson RA, EC Buck, J Chun, RC Daniel, DL Herting, ES Ilton, GJ Lumetta, and SB Clark. 2018. "Review of the Scientific Understanding of Radioactive Waste at the U. S. DOE Hanford Site." Environmental Science & Technology 52(2):381-396. doi:10.1021/acs.est.7b04077